CINCH NucWik

User Tools

Site Tools

You are here: NucWik » RoboLab Remote Controlled Experiments » RoboLab: Neutron Activation of Silver - Experimental Procedure

Sidebar

CINCH project

NRC Network

CINCH Hub

remote_control_experiments:neutron_activation_of_ag

Differences

This shows you the differences between two versions of the page.

Link to this comparison view

Both sides previous revision Previous revision
Next revision 		Previous revision
remote_control_experiments:neutron_activation_of_ag [2023-10-03 11:26]
Jon Peter Omtvedt 		remote_control_experiments:neutron_activation_of_ag [2023-10-03 12:09] (current)
Jon Peter Omtvedt
Line 75: Line 75:
 {{:remote_control_experiments:robolabnaacontrolscreen.jpg?600}}\\ {{:remote_control_experiments:robolabnaacontrolscreen.jpg?600}}\\
  
-(click on the picture to see a larger version.) You must preset the duration for all the measurement periods (rows in the table) before you perform irradiations. In the beginning you want short intervals to follow the rapid decay, then you switch to longer intervals. We suggest 5x 20 sec followed by 100 sec intervals for the remaining time periods. You should continue measuring until the number of counts fluctuate around the background radiation level in the lab. +(click on the picture to see a larger version.) You must preset the duration for all the measurement periods (rows in the table) before you perform irradiations. In the beginning you want short intervals to follow the rapid decay, then you switch to longer intervals. We suggest 5x 20 sec followed by 100 sec intervals for the remaining time periods (this will be the defaults when you start up RoboLab). 
  
 +//Background Measurement//\\
 +For each irradiation you do, you should continue measuring until the number of counts fluctuate around the background radiation level in the lab. Therefore, before you start irradiations you should perform a background measurement. The easiest way to do this is to select e.g. a 300 sec preset duration for the first row in the table and start counting. Once the system finishes with the first measurement and start measuring counts for the second row in the table you can stop and write down the number of counts obtained for the first row. You then divide the counts by the duration to obtain your background count rate in cps (counts per second). 
  
-. for the short  This will provi with the  and measure the resulting decay curves of the two silver isotopes. +//Performing irradiations//\\ 
-It is important that you let the silver decay before you perform the subsequent irradiations, possible to use a system such as RoboLab.\\+Make sure you have reset the counting duration after the background measurement to whatever you have selected (probably 20 sec). You can now start performing irradiations. Select a preset time in the irradiation control box (to the left) and push the start irradiation button. In the video feed you will see that the slide with the silver disc disappears - it is sent to the neutron irradiation position on the other side of the concrete wall. There is a sensor inside that keeps track of the actual irradiation time. There is also an irradiation indicator light on the control panel. As soon as you see the slide back on top of the detector you start counting by clicking the start counting button (make sure you have cleared the counters before you started the irradiation). The system will now automatically fill in counts in the table and update the start time for each individual measurement interval. Let it run until you are certain you are only measuring background. Write down all the results before clearing the counter for the next irradiation. 
  
-\\  +Repeat the procedure above for all your irradiation times. This will conclude the experimental part of your experiment. Remember that if you start an irradiation that somehow did not work out as expected (e.g. wrong preset time) you //must// wait for the induced radioactivity in the silver disk to die out before making a new attempt. Otherwise the measured activity is not representative for the selected irradiation time. 
  
-__How to measure the Decay of n-activated Ag__\\+==== Plotting the Measured Data ==== 
 +Use a high-quality data plotting and fitting program (e.g. Origin) to plot and analyze the data. If you use the plotting program to also "fit" the data, i.e. find parameters for a two-component decay curve that matches your measurement points in the best possible way, the fitting algorithm must take the uncertainty into account (do not use Excel unless you know how to use the "solver" add-on to do this correctly), otherwise you will get wrong results.
  
-//Introduction//\\ +Notice that you always shall use the 1/3 of the time into each measurement as the "middle time point". This is due to decay - after 1/3 of the time you will have equally many counts before and after the 1/3 point (i.e. it is the "middle point".
-For this part of the exercise, you will use a NaI detector connected to a Multi-Channel Analyzer (MCA) to determine the disintegration rate of the n-activated silver.+
  
-//Principle//\\ +For each irradiation interval plot your data as follows:  
-This description assumes you have the Maestro MCA software from ORTEC. If you are using an alternative system, you will have to consult the manual to figure out how to use it. The procedure should not be very different, though.\\ +  * For each data point calculate the net count (gross count minus background count), the uncertainty of the net count (based on uncertainty of both the gross count and the background count).  
-We want to make successive 20-s measurements followed by 120-s ones to determine the half-life curve of the silver isotopes. This can be done manually by successive starting-waiting-stopping-saving-clearing operations.\\ +  * Enter your data in a table ("worksheet" if you use Origin) or whatever your plotting program uses: Include measurement time (relative to end of irradiation) as x-value, the net count as y-value, and the uncertainty as y-error. 
-However, with a modern system this tiresome procedure can be automated: In Maestro jargon you do this by preparing a job-description file (it would be called a script file or batch file in most other software). This file contain all the instructions you would have to execute, but can be simplified by using the built-in loop structure. Furthermore, once running, it will execute the correct commands at exactly the right time.\\ +  * Plot the data - does it look OK? If not, find the error. Your measurement points should lie on a line that gradually decay in a smooth way (within statistical uncertainty). 
-Since the commands execute very rapidly, you will also be able to spend practically all the time actually counting, something witch is not possible if you are doing everything manually.+
  
-Job-description file: +==== Deconvoluting the Decay Curve ====
-  set_preset_real 20\\ +
-  loop 7\\ +
-  clear\\ +
-  start\\ +
-  wait\\ +
-  save m:\spectra\KJM5911_D130_A???.chn\\ +
-  end_loop\\+
  
-  set_preset_real 120\\ +Notice: The steps indicated below is not very detailed. We assume that you have a teacher physically present that can help you use whatever software and method he/she has prepared for this exercise. How your teaching institution use the data measured with this RoboLab will vary. They might also have provided a more detailed description than what is provided below. 
-  loop 7\\ +
-  clear\\ +
-  start\\ +
-  wait\\ +
-  save m:\spectra\KJM5911_D130_B???.chn\\ +
-  end_loop\\ +
- +
-  set_preset_real 300\\ +
-  clear\\ +
-  start\\ +
-  wait\\ +
-  save m:\spectra\KJM5911_D130_Background.chn\\ +
- +
-This job-file will perform 8 20-s measurement, then 8 120-s measurements and finally a 5-min background measurement. +
-\\ +
- +
-//Procedure//\\ +
-The MCA will save spectra containing counts vs. energy. The two interesting gamma-rays from the n-activated silver will overlap and you will not be able to differentiate between them in the NaI spectra. Thus, we will simply use the gross counts and subtract the background as if we had used a simple counter.\\ +
-The procedure for measuring each irradiated silver disk is as follows: +
-  -Measure a background spectrum for as long as possible if you have not already done this. +
-  -Get the irradiated silver disk and put it as quickly as possible on top of the detector. +
-  -Start the job-file and note down the time between end-of-irradiation and starting the job-file. +
-  -Now, sit back and relax! Alternatively (better), if the job-file is saving spectra to a network disk, you can analyze the spectra as they are produced (using another pc which can read the same disk). +
-  -When the job-file finishes, repeat the measurement for the different irradiation times (irradiation times = 12, 24, 48, 72, and 144 s). (Remember to rename or move your spectra, otherwise they will be deleted or the job-file stops.) +
- +
-From the spectra you should get the following data (by opening each spectrum in Maestro): The measurement start time and the gross count (total number of counts in the spectrum). Use the "sum" command to get the total number of counts (the spectrum must contain no region-of-interest markings).\\  +
- +
-Alternative procedure: Select the relevant spectrum region with the photo-peaks and only use the integrals under this (double-)peak for analyzing the data. +
- +
-\\ +
-\\  +
-__Analyzing a two-component Decay curve__\\ +
-\\  +
-Use a high-quality data plotting and fitting program (e.g. Origin) to analyze the data. The fitting ''must'' take the uncertainty into account (do not use Excel), otherwise you will get the wrong result. +
-Notice that you always shall use the 1/3 of the time into each measurement as the "middle time point". This is due to decay - after 1/3 of the time you will have equally many counts before and after the 1/3 point (i.e. it is the "middle point". +
-  -For each data point calculate the net count (gross count - background count), the uncertainty of the net count (based on uncertainty of both the gross count and the background count). You might want to use e.g. MS Excel or similar for doing this. +
-  -Enter your data in a table ("worksheet" in Origin jargon): Include measurement time (relative to end of irradiation) as x-value, the net count as y-value, and the uncertainty as y-error. +
-  -Plot the data - does it look OK? +
-\\ +
  
 //Manual Method//\\ //Manual Method//\\
Line 153: Line 108:
  
 //Automated Method//\\ //Automated Method//\\
-Use the Origin data-fitting functionality to determine the measured half-life of both components simultaneously. +Use your plotting programs fitting functionality to determine the measured half-life of both decay components simultaneously. It is also possible to fit the background level automatically. If so, it should not deviate much from the background you measured (this typically happen if you have terminated your decay measurement too early). 
-"Alternative/Extra": Plot the gross counts instead of the net counts and ask Origin to fit both the background and the two components at the same time. +
 \\  \\ 
  
-__Analyzing the Production Curve of n-activated Ag__\\ +==== Analyzing the Production Curve of n-activated Ag ====
  
-From analyzing the decay curves for the different irradiation times (12, 24, 48, 72, and 144 s) you should have five R<sub>0</sub> values for each of the isotopes:+From analyzing the decay curves for the different irradiation times (e.g. 12, 24, 48, 72, and 144 s) you should have a corresponding number of R<sub>0</sub> values for each of the isotopes:
  
-  -Plot the R<sub>0</sub> values as a function of irradiation time (use Origin or similar software). +  * Plot the R<sub>0</sub> values as a function of irradiation time (use Origin or similar software). 
-  -Assume that the R<sub>0</sub> for the <sup>110</sup>Ag irradiation is exact. Use this value to determine the product of the detector-efficiency and neutron flux. In the following, use this value as "true" whenever you need the product. +  * Assume that the R<sub>0</sub> for the <sup>110</sup>Ag irradiation is exact. Use this value to determine the product of the detector-efficiency and neutron flux. In the following, use this value as "true" whenever you need the product. 
-  -Use the weight of the silver plate to determine the number of target atoms (silver atoms). +  * Use the weight of the silver plate to determine the number of target atoms (silver atoms). 
-  -Now calculate the ''theoretical'' points for the nine other R<sub>0</sub> points. +  * Now calculate the ''theoretical'' points for the nine other R<sub>0</sub> points. 
-  -How does your theoretical and experimentally measured points agree? +  * How does your theoretical and experimentally measured points agree?
- +
-\\ +
  
 +Notice: Again, the above description is not very detailed. Your teacher will instruct how your are supposed to do this for your particular exercise with the RoboLab system. 
  
-==== Questions for the students ==== 
-Use the cross-sections from the nuclear chart, the half life and a thermal neutron-flux of 2*103 n/cm<sup>2</sup>s to estimate the relative amount you will produce for a 144 s irradiation. Which nuclei will be dominant? 
-Determine what kind of gamma radiation to expect from the silver isotopes produced in the irradiation and their associated relative intensity (e.g. from Berkeley/Lund database). 
  
remote_control_experiments/neutron_activation_of_ag.1696325211.txt.gz · Last modified: 2023-10-03 11:26 by Jon Peter Omtvedt

Page Tools

A-CINCH Consortium

email: mst@evalion.cz | tel: +420 224 358 331 | Copyright © 2021 A-CINCH
This project has received funding from the Euratom research and training programme 2019–2020 under grant agreement No. 945301.